Don Messick
Papa Smurf (voice) (422 eps)
Lucille Bliss
Smurfette (voice) (422 eps)
Frank Welker
Hefty Smurf (voice) (422 eps)
Michael Bell
Handy Smurf (voice) (422 eps)
June Foray
Jokey Smurf (voice) (422 eps)
Paul Winchell
Gargamel (voice) (422 eps)
Danny Goldman
Brainy Smurf (voice) (422 eps)
Hamilton Camp
Greedy Smurf (voice) (422 eps)
William Callaway
Clumsy Smurf (voice) (422 eps)