Hank Azaria
Gargamel (voice)
Melissa Sturm
Smurfette (voice)
Frank Welker
Azrael (voice)
Anton Yelchin
Clumsy Smurf (voice)
Tom Kane
Narrator Smurf (voice)
Alan Cumming
Gutsy Smurf (voice)
Fred Armisen
Brainy Smurf (voice)
Jack Angel
Papa Smurf (voice)
Adam Wylie
Panicky Smurf (voice)
John Oliver
Vanity Smurf (voice)
Gary Basaraba
Hefty Smurf (voice)