Jack Angel
Papa Smurf (Voice)
Fred Armisen
Brainy (Voice)
Hank Azaria
Gargamel (Voice)
Gary Basaraba
Hefty (Voice)
George Lopez
Grouchy (Voice)
Melissa Sturm
Smurfette (Voice)
Anton Yelchin
Clumsy (Voice)
Frank Welker
Azrael (voice)